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Ozawa, Takayuki; Hirooka, Shun; Kato, Masato; Novascone, S.*; Medvedev, P.*
Journal of Nuclear Materials, 553, p.153038_1 - 153038_16, 2021/09
Times Cited Count：4 Percentile：56.94(Materials Science, Multidisciplinary)To evaluate the O/M dependence of pore migration regarding fuel restructuring at the beginning of irradiation, we are developing BISON for MOX in cooperation with INL and have installed pore migration model considering vapor pressure of vapor species and thermal conductivity for MOX. The O/M dependence of fuel restructuring observed in MA-bearing MOX irradiation experiment in Joyo was evaluated by the 2-dimensional analyses. Four MA-bearing MOX pins with different O/M ratio and pellet/cladding gap size were irradiated in Joyo B14 experiment. Remarkable restructuring of stoichiometric MA-bearing MOX fuels was observed in PIE, and could be evaluated by considering the influence of O/M ratio on vapor pressure. Also, a central void assumes to move toward wide-gap side when the pellet eccentricity taking place, but 2-dimentional analyses on pellet transverse section revealed that the central void formation observed in PIE would be inconsistent with a direction of the pellet eccentricity.
Wakaida, Ikuo; Akaoka, Katsuaki; Miyabe, Masabumi; Khumaeni, A.; Oba, Hironori; Saeki, Morihisa; Ito, Chikara; Otobe, Haruyoshi; Kato, Masaaki
no journal, ,
In the next generation nuclear fuel cycle, low-decontaminated fuel with TRU will be strongly required, and convenience, quick analytical techniques will be necessary. Simultaneous analysis of element and isotope by the combination of Laser Induced Breakdown Spectroscopy (LIBS) and Ablation Resonance Absorption Spectroscopy was demonstrated. For elemental analysis, detection lower limit of 1000 ppm of Pu in U oxide and relative error under 5% have been obtained within 5 min. For isotope analysis, 
Pu and 
Pu have been observed completely separated, and detection lower limit of several 10 ppm and error under 1% have been accomplished. A simple antenna coupled microwave assisted LIBS was performed and the enhancement of emission intensity of several 10 times was demonstrated. For liquid sample, ultra-thin laminate flow as the laser focused target was accomplished high sensitivity of ppb. For in-situ monitoring, Optical Fiber LIBS Probe by radiation resistant optical fiber is under construction.
Maeda, Seiichiro
no journal, ,
The uranium-plutonium mixed oxide (MOX) fuel bearing several percent minor actinides is adopted as the fast reactor fuel to reduce the high level radioactive waste volume and its toxicities. Their physical properties such as melting points and thermal conductivities are investigated symmetrically. It is getting clear that the effect of MA bearing is not so significant. The MOX fuel pins including up to 5% of Am were irradiated in Joyo to confirm their irradiation performance. Some types of irradiation experiments using MA-MOX fuels are planned after Joyo restart. The obtained data will contribute to develop fuel pin performance codes for MA-MOX fuels. SmART (Small Amount of Reuse Fuel Test) cycle program is in progress to demonstrate MA recycles starting from FR spent fuels. Furthermore, long life cladding with ODS steel is under development to enhance the transmutation efficiency of MA in one cycle. Thus, R&Ds in FR systems advances steadily to solve the waste issue.
Ozawa, Takayuki; Hirooka, Shun; Kato, Masato; Verdolin, F.*; Novascone, S.*
no journal, ,
3-dimensional analysis code BISON-MOX to be applied for the irradiation behavior of MOX fuels is being developed by installing MOX fuel properties and analysis models to BISON, which has been developed in INL. Applying the thermal conductivity of MOX fuel and the pore migration model based on vapor pressure of vapor species, the O/M dependence of fuel restructuring observed in MA-bearing MOX fuels irradiation in Joyo were evaluated by 2-dimensional analyses with BISON-MOX.
Ozawa, Takayuki; Hirooka, Shun; Kato, Masato; Novascone, S.*; Medvedev, P.*
no journal, ,
To evaluate the O/M dependence of pore migration regarding fuel restructuring at the beginning of irradiation, we are developing BISON for MOX in cooperation with INL and have installed pore migration model considering vapor pressure of vapor species and thermal conductivity for MOX. The O/M dependence of fuel restructuring observed in MA-bearing MOX irradiation experiment in Joyo was evaluated by the 2-dimensional analyses. Four MA-bearing MOX pins with different O/M ratio and pellet/cladding gap size were irradiated in Joyo B14 experiment. Remarkable restructuring of stoichiometric MA-bearing MOX fuels was observed in PIE, and could be evaluated by considering the influence of O/M ratio on vapor pressure. Also, a central void assumes to move toward wide-gap side when the pellet eccentricity taking place, but 2-dimentional analyses on pellet transverse section revealed that the central void formation observed in PIE would be inconsistent with a direction of the pellet eccentricity.
Onishi, Takashi; Morishita, Kazuki; Watanabe, Masashi; Yokoyama, Keisuke; Kato, Masato
no journal, ,
no abstracts in English
